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Construction of TiO2 on cotton straw deposited on g-C3N4 heterojunction to improve the photocatalytic degradation activity of methylene blue and tetracycline

DIAMOND AND RELATED MATERIALS [2024]
Tianyi Cui, Yuan Zhang, Mingxia Tian, Yumin Yan, Guyu Zhang, Tao Zhang, Jianbo Zhao, Jianhui Jiang
ABSTRACT

In this study, agricultural waste cotton stalk was used as biomass carbon source, calcined with TiO 2 at a high temperature, deposited in a TiO 2 lattice, and used as an electron acceptor to inhibit photogenerated electron recombination. Subsequently, it underwent secondary calcination with g-C 3 N 4 to form a C-TiO 2 /g-C 3 N 4 composite catalyst. Experimental results showed that the coupling of carbon-doped TiO 2 and g-C 3 N 4 accelerated photogenerated electron–hole pairs pair migration, effectively inhibited the recombination of photogenerated carriers, and thus improved the removal efficiency of methylene blue (MB) and tetracycline hydrochloride (TC). Upon irradiation with a 500 W xenon lamp, the degradation rates of MB and TC achieved were 92.6 % and 95.3 % in 90 min, respectively.

MATERIALS

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