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Carbon dots induced in-situ formation of porous europium micro-networks with enhanced photocatalysis

JOURNAL OF COLLOID AND INTERFACE SCIENCE [2022]
Yue Wang, Bin-Bin Chen, Ya-Ting Gao, Lei Jiang, Jian Lv, Shuai Chang, Ruo-Can Qian, Da-Wei Li
ABSTRACT

Excellent photocatalysts are highly desirable for clean energy and pollutant treatment. Carbon dots (CDs)-based composite photocatalysts have been widely studied and utilized in catalytic fields. However, the preparation of the photocatalysts with high catalytic activity still faces a great challenge. Herein, white-light-driven CDs-based porous europium micro-networks (CDs@P-Eu-MNs) composite photocatalysts are prepared by a facile in-situ growth strategy. CDs can affect the morphology and produce a large number of porous structures of CDs@P-Eu-MNs. Importantly, the introduction of CDs not only increases the light absorption, but also promotes the separation of photogenerated charge carriers, and thus improve photocatalytic performance of CDs@P-Eu-MNs composites. CDs@P-Eu-MNs show the highest photocurrent density, which can be used for the highly-efficient photodegradation of rhodamine 6G dyes with almost 95% degradation rate under low power white light (20 W) without any radical generating agents such as H 2 O 2 . Therefore, this new and efficient CDs@P-Eu-MNs photocatalyst will have a great application prospect in water pollution treatment.

MATERIALS

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