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Facile fabrication of biomass chitosan-derived magnetic carbon aerogels as multifunctional and high-efficiency electromagnetic wave absorption materials

CARBON [2024]
Shijie Wang, Xue Zhang, Yunxiang Tang, Shuyan Hao, Sinan Zheng, Jing Qiao, Zhou Wang, Lili Wu, Jiurong Liu, Fenglong Wang
ABSTRACT

Biomass chitosan-derived porous carbon-based materials take the advantage of light weight, adjustable intrinsic conductivity, and environmental friendliness, attracting more attention in the field of electromagnetic compatibility. However, exploring a facile fabrication method to achieve rational structure design and electrical-magnetic coupling for electromagnetic absorption performance enhancement still remains challenging. Here, a unique honeycomb-like porous cobalt/carbon aerogel is fabricated through the directional freezing-drying and carbonization process, and abundant and even-distributed cobalt particles in-situ grow on the carbon skeletons. The aerogel exhibits an impressive electromagnetic wave absorption performance of a −75.8-dB absorption intensity and a −256.9-dB mm −1 specific reflection loss at a low filling content (10%), as well as an 8.53-GHz effective absorption bandwidth. Besides, the aerogel also demonstrates classy radar stealth and thermal insulation performance. The eco-friendly, easily fabricated, and high-performance cobalt/carbon aerogel suggests broad application prospects for electromagnetic compatibility and protection, thermal management, and multifarious electron devices.

MATERIALS

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